113199
PTDC/FIS/113199/2009
FCT - Fundação para a Ciência e a Tecnologia, I.P.
Portugal
5876-PPCDTI
141,247.00 €
2011-02-01
2014-07-31
Semiconductor quantum dots (QDs), often referred to as "artificial atoms", have discrete energy levels that can be tuned by changing the QD size and shape. The existence of zero-dimensional states in QDs has been proved by high spectrally and spatially resolved photoluminescence (PL) studies Empedocles et al. (1996); Grundmann et al. (1995). Semiconductor QDs can be divided into two types, (1) epitaxially grown...
It is shown that quantitative information on spatial correlations in a system of polarizable particles can be extracted directly from its experimentally measurable optical spectra. For a collection of metallic nanoparticles (NPs), it is demonstrated that the degree of shortrange correlation in NP’s positions can be evaluated by an appropriate numerical analysis of the extinction spectrum in the surface plasmon ...
Dissertação de mestrado em Química Medicinal; Colloidal Quantum Dots (QDs) are promising systems for optoelectronic and biotechnology applications, since they have a higher photostability compared to classical fluorophores and their absorption and emission properties can be tuned during synthesis. Among the numerous alternative nanometer building blocks, colloidal QDs are of particular interest in the formation...
Comunicação Oral Convidada.; A soft method for the production of CdSe and CdSe/Zns quantum dots is presented, as well as the main experimental results.; Fundação para a Ciência e a Tecnologia (FCT), FEDER and QREN for financial support to CFUM [Strategic Project PEst-C/FIS/UI0607/2011 (F-COMP-01-0124-FEDER-022711)] and to the research project PTDC/FIS/113199/2009 also financed by COMPETE/QREN/EU.
We present a theoretical description of Bogolyubov-type excitations of exciton-polariton Bose-Einstein condensates (BECs) in semiconductor microcavities. For a typical two-dimensional (2D) BEC we focus on two limiting cases, the weak-and strong-coupling regimes, where a perturbation theory and the Thomas-Fermi approximation, respectively, are valid. We calculate integrated scattering intensity spectra for probi...
"Published in SPIE Proceedings Vol. 9286"; We present a flexible fluorescence lifetime imaging device which can be employed to scan large sample areas with a spatial resolution adjustable from many micrometers down to sub-micrometers and a temporal resolution of 20 picoseconds. Several different applications of the system will be presented including protein microarrays analysis, the scanning of historical sampl...
The band structure and the optical conductivity of an ABA (Bernal-type) stacked graphene trilayer are calculated. It is shown that, under appropriate doping, a strong resonant peak develops in the optical conductivity, located at the frequency corresponding to approximately 1.4 times the interlayer hopping energy and caused by the 'nesting' of two nearly parabolic bands in the electronic spectrum. The intensity...
We theoretically investigate the optical response of ensembles of polarizable metallic nanoparticles (NPs) that form (1) submonolayer films of particles adsorbed on a dielectric substrate, considered as two-dimensional (2-D) systems, and (2) thin three-dimensional (3-D) films, where NPs are embedded in a dielectric matrix. For system (1), the effect of NPs’ distance to the substrate is taken into account. In bo...
The exceptional properties of localised surface plasmons (LSPs), such as local field enhancement and confinement effects, resonant behavior, make them ideal candidates to control the emission of luminescent nanoparticles. In the present work, we investigated the LSP effect on the steady-state and time-resolved emission properties of quantum dots (QDs) by organizing the dots into self-assembled dendrite structur...
We fabricated dendrite-type superstructures of fractal dimension consisting of CdSe/ZnS & CdTe capped nanodots. These structures were studied using microscopic fluorescence intensity imaging as well as spectral and lifetime mapping.; FCT Concurso "Ciência 2007"; MAP-Fis Doctoral Programme (Doutoramento FCT); info:eu-repo/semantics/publishedVersion
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